Superdiffusion and heterogeneous dynamics in liquid crystals by microrheology García Daza, Fabián Puertas, Antonio M. Cuetos, Alejandro Patti, Alessandro Liquid Crystals Colloids Brownian motion Microrheology Monte Carlo simulation F.A.G.D. and A.P. acknowledge a María Zambrano fellowship, funded by the NextGenerationEU/PRTR program of the European Union, the Plan de Recuperación, Transformación y Resiliencia, and the Ministerio de Universidades. A.C., A.M.P. and A.P. acknowledge, respectively, grants PID2021-126121NB-I00, PID2021-127836NB-I00 and PID2022-136540NB-I00 awarded by MICIU/AEI/10.13039/501100011033 and ERDF A way of making Europe. A.P. also acknowledges grant P21_00015 funded by Junta de Andalucía - Consejería de Universidad, Investigación e Innovación. Microrheology (MR) has emerged as a powerful tool for unraveling the intricate local viscoelastic properties of various soft materials. By tracking the free (passive MR) or forced (active MR) diffusion of a tracer, valuable insights into the mechanical characteristics of the host system can be obtained. In this study, we investigate the forced diffusion of a spherical tracer within isotropic and smectic liquid crystal phases of hard rod-like particles. Our findings reveal superdiffusive behaviour induced by external forces, particularly pronounced when these are aligned parallel to the nematic director. Analysis of dynamical susceptibility unveils heterogeneities strongly correlated with the magnitude and orientation of applied forces, highlighting the system’s critical dependence on structural ordering. Intriguingly, we observe that tracer superdiffusion, driven by external forces and evident across all relevant system directions, does not demonstrate a strong correlation with resulting dynamical heterogeneities. 2024-12-13T11:13:37Z 2024-12-13T11:13:37Z 2024 journal article Published version: García Daza, F. A., Puertas, A. M., Cuetos, A., & Patti, A. (2024). Superdiffusion and heterogeneous dynamics in liquid crystals by microrheology. Molecular Physics. https://doi.org/10.1080/00268976.2024.2396546 https://hdl.handle.net/10481/97992 10.1080/00268976.2024.2396546 eng http://creativecommons.org/licenses/by-nc-nd/3.0/ open access Creative Commons Attribution-NonCommercial-NoDerivs 3.0 License Taylor and Francis