Self-assembly in magnetic supramolecular hydrogels Gila Vilchez, Cristina Rodríguez Arco, Laura Mañas Torres, María del Carmen Álvarez de Cienfuegos, Luis López López, Modesto Torcuato Magnetic hydrogels Supramolecular hydrogels Magnetic nanoparticles Smart materials Magneto-responsiveness Drug delivery Tissue engineering Most recent advances in the synthesis of supramolecular hydrogels based on low molecular weight gelators (LMWGs) have focused on the development of novel hybrid hydrogels, combining LMWGs and different additives. The dynamic nature of the noncovalent interactions of supramolecular hydrogels, together with the specific properties of the additives included in the formulation, allow these novel hybrid hydrogels to present interesting features, such as stimuli-responsiveness, gel-sol reversibility, self-healing and thixotropy, which make them very appealing for multiple biomedical and biotechnological applications. In particular, the inclusion of magnetic nanoparticles in the hydrogel matrix results in magnetic hydrogels, a particular type of stimuli-responsive materials that respond to applied magnetic fields. This review focuses on the recent advances in the development of magnetic supramolecular hydrogels, with special emphasis in the role of the magnetic nanoparticles in the self-assembly process, as well as in the exciting applications of these materials. 2023-02-06T11:08:51Z 2023-02-06T11:08:51Z 2022-12 info:eu-repo/semantics/article C. Gila-Vilchez et al. Current Opinion in Colloid & Interface Science Volume 62, December 2022, 101644 https://hdl.handle.net/10481/79679 10.1016/j.cocis.2022.101644 eng http://creativecommons.org/licenses/by-nc-nd/3.0/ info:eu-repo/semantics/openAccess Creative Commons Attribution-NonCommercial-NoDerivs 3.0 License