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dc.contributor.authorYus-Díez, Jesús
dc.contributor.authorTitos Vela, Gloria
dc.identifier.citationYus-Díez, J., Ealo, M., Pandolfi, M., Perez, N., Titos, G., Močnik, G., Querol, X., and Alastuey, A.: Aircraft vertical profiles during summertime regional and Saharan dust scenarios over the north-western Mediterranean basin: aerosol optical and physical properties, Atmos. Chem. Phys., 21, 431–455, []es_ES
dc.descriptionWe acknowledge support of the publication fee by the CSIC Open Access Publication Support Initiative through its Unit of Information Resources for Research (URICI).es_ES
dc.descriptionThis research has been supported by the Generalitat de Catalunya, Agencia de Gestio d'Ajuts Universitaris i de Recerca (grant nos. AGAUR 2014 SGR33 and AGAUR 2017 SGR41); the Ministerio de Economia, Industria y Competitividad, Gobierno de Espana (HOUSE; grant no. CGL2016-78594-R); and the European Commission's Horizon 2020 Framework Programme (ACTRIS-2; grant no. 654109).es_ES
dc.description.abstractAccurate measurements of the horizontal and vertical distribution of atmospheric aerosol particle optical properties are key for a better understanding of their impact on the climate. Here we present the results of a measurement campaign based on instrumented flights over north-eastern Spain. We measured vertical profiles of size-segregated atmospheric particulate matter (PM) mass concentrations and multi-wavelength scattering and absorption coefficients in the western Mediterranean basin (WMB). The campaign took place during typical summer conditions, characterized by the development of a vertical multi-layer structure, under both summer regional pollution episodes (REGs) and Saharan dust events (SDEs). REG patterns in the region form under high insolation and scarce precipitation in summer, favouring layering of highly aged fine-PM strata in the lower few kma.s.l. The REG scenario prevailed during the entire measurement campaign. Additionally, African dust outbreaks and plumes from northern African wildfires influenced the study area. The vertical profiles of climate-relevant intensive optical parameters such as single-scattering albedo (SSA); the asymmetry parameter (g); scattering, absorption and SSA Ångström exponents (SAE, AAE and SSAAE); and PM mass scattering and absorption cross sections (MSC and MAC) were derived from the measurements. Moreover, we compared the aircraft measurements with those performed at two GAW–ACTRIS (Global Atmosphere Watch–Aerosol, Clouds and Trace Gases) surface measurement stations located in north-eastern Spain, namely Montseny (MSY; regional background) and Montsec d'Ares (MSA; remote site). Airborne in situ measurements and ceilometer ground-based remote measurements identified aerosol air masses at altitudes up to more than 3.5 kma.s.l. The vertical profiles of the optical properties markedly changed according to the prevailing atmospheric scenarios. During SDE the SAE was low along the profiles, reaching values < 1.0 in the dust layers. Correspondingly, SSAAE was negative, and AAE reached values up to 2.0–2.5, as a consequence of the UV absorption increased by the presence of the coarse dust particles. During REG, the SAE increased to > 2.0, and the asymmetry parameter g was rather low (0.5–0.6) due to the prevalence of fine PM, which was characterized by an AAE close to 1.0, suggesting a fossil fuel combustion origin. During REG, some of the layers featured larger AAE (> 1.5), relatively low SSA at 525 nm (< 0.85) and high MSC (> 9 m2 g−1) and were associated with the influence of PM from wildfires. Overall, the SSA and MSC near the ground ranged around 0.85 and 3 m2 g−1, respectively, and increased at higher altitudes, reaching values above 0.95 and up to 9 m2 g−1. The PM, MSC and MAC were on average larger during REG compared to SDE due to the larger scattering and absorption efficiency of fine PM compared with dust. The SSA and MSC had quite similar vertical profiles and often both increased with height indicating the progressive shift toward PM with a larger scattering efficiency with altitude. This study contributes to our understanding of regional-aerosol vertical distribution and optical properties in the WMB, and the results will be useful for improving future climate projections and remote sensing or satellite retrieval algorithms.es_ES
dc.description.sponsorshipGeneralitat de Catalunya, Agencia de Gestio d'Ajuts Universitaris i de Recerca AGAUR 2014 SGR33 AGAUR 2017 SGR41es_ES
dc.description.sponsorshipMinisterio de Economia, Industria y Competitividad, Gobierno de Espana (HOUSE) CGL2016-78594-Res_ES
dc.description.sponsorshipEuropean Commission's Horizon 2020 Framework Programme (ACTRIS-2) 654109es_ES
dc.publisherCopernicus Publications; European Geosciences Uniones_ES
dc.rightsAtribución 3.0 España*
dc.titleAircraft vertical profiles during summertime regional and Saharan dust scenarios over the north-western Mediterranean basin: aerosol optical and physical propertieses_ES
dc.relation.projectIDinfo:eu-repo/grantAgreement/EC/H2020/654109 ACTRIS-2es_ES

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