# Title: Rotational excitation of molecules in the regime of strong ro-vibrational coupling: # Comparison between an optical centrifuge and a transform-limited pulse # Authors: J. M. García-Garrido, V. Milner, C. P. Koch & R. González-Férez # DOI: https://doi.org/10.1039/D5CP02931G # Data from fig. 6 # Gaussian pulse parameters: # I^G_0=1E12 W/cm^2 # sigma=0.142440 ps # t_g=0.670841 ps # t_G=1.341682 ps # # N v |C_{v,N}(0.533ps)|^2 |C_{v,N}(0.672ps)|^2 |C_{v,N}(0.790ps)|^2 |C_{v,N}(tf)|^2 0 0 1.1180e-14 2.4560e-14 7.3030e-11 2.0810e-10 2 0 3.0930e-13 1.7730e-12 3.8040e-10 1.0300e-09 4 0 6.7030e-13 1.0380e-12 6.4600e-10 1.8150e-09 6 0 3.8480e-13 2.8940e-12 9.0680e-10 2.5390e-09 8 0 1.0200e-13 2.7700e-12 1.1010e-09 3.1640e-09 10 0 1.5450e-14 2.0060e-12 1.2500e-09 3.6960e-09 12 0 1.5240e-15 4.1630e-12 1.3550e-09 4.0720e-09 14 0 9.7150e-17 2.2640e-12 1.3650e-09 4.3410e-09 16 0 6.1570e-18 1.4530e-12 1.3600e-09 4.4320e-09 18 0 5.7220e-20 3.0020e-12 1.2730e-09 4.3980e-09 20 0 2.2290e-20 2.8470e-12 1.1470e-09 4.2300e-09 22 0 2.7410e-20 1.3360e-12 1.0130e-09 3.9220e-09 24 0 1.3170e-19 3.2440e-13 8.4280e-10 3.5440e-09 26 0 6.2300e-20 2.9650e-14 6.6950e-10 3.0830e-09 28 0 3.6560e-21 1.4830e-15 5.1760e-10 2.5780e-09 30 0 8.7330e-20 5.6920e-15 3.8250e-10 2.0880e-09 32 0 1.1280e-19 4.1330e-15 2.6560e-10 1.6140e-09 34 0 6.7600e-20 1.6910e-15 1.7380e-10 1.1840e-09 36 0 5.2900e-21 4.6920e-16 1.0970e-10 8.3400e-10 38 0 4.7070e-21 1.0460e-16 6.9220e-11 5.6020e-10 40 0 1.4780e-19 1.9490e-17 4.3830e-11 3.5120e-10 42 0 6.3130e-20 1.4970e-18 2.6500e-11 2.0590e-10 44 0 1.0180e-20 2.3640e-19 1.4430e-11 1.1690e-10 46 0 3.7790e-20 1.1440e-19 6.8400e-12 6.5900e-11 48 0 1.1710e-19 1.5050e-21 2.7920e-12 3.6180e-11 50 0 6.4660e-20 1.1750e-19 9.8070e-13 1.8450e-11 52 0 5.7890e-20 3.4160e-20 2.9910e-13 8.4020e-12 54 0 4.2540e-20 1.3050e-21 7.9530e-14 3.3580e-12 56 0 2.1480e-20 5.7930e-20 1.8610e-14 1.1730e-12 58 0 1.0980e-19 2.9220e-20 3.8380e-15 3.5770e-13 60 0 1.5250e-19 7.7310e-21 7.1970e-16 9.6280e-14 62 0 2.7200e-20 1.2730e-19 1.1380e-16 2.2700e-14 64 0 7.2510e-20 7.8240e-20 1.9300e-17 4.8140e-15 66 0 5.8320e-20 5.3860e-20 1.6590e-18 8.8210e-16 68 0 7.5760e-20 8.3560e-20 6.2270e-19 1.4970e-16 70 0 1.1990e-20 4.6460e-20 4.5380e-20 2.1740e-17 72 0 2.5860e-20 3.2080e-20 6.8450e-20 2.6800e-18 74 0 1.3950e-20 1.0520e-19 8.0800e-20 5.3030e-19 76 0 2.7620e-20 1.0430e-20 1.9960e-19 1.4940e-19 78 0 5.6650e-20 8.4000e-20 2.8310e-21 2.1680e-19 0 1 3.1330e-13 3.0930e-12 2.0320e-09 5.5820e-09 2 1 1.9590e-12 3.1230e-12 9.6490e-09 2.7670e-08 4 1 4.4950e-12 8.7710e-12 1.7200e-08 4.8830e-08 6 1 2.2880e-12 1.0730e-11 2.3320e-08 6.8160e-08 8 1 5.4030e-13 3.5140e-12 2.8740e-08 8.5410e-08 10 1 7.5410e-14 1.3940e-11 3.2460e-08 9.9190e-08 12 1 7.0280e-15 4.9820e-12 3.4490e-08 1.1020e-07 14 1 4.6250e-16 1.1390e-12 3.5390e-08 1.1660e-07 16 1 2.3510e-17 6.1960e-12 3.4060e-08 1.1980e-07 18 1 6.6730e-19 7.8560e-12 3.1910e-08 1.1870e-07 20 1 3.7560e-21 6.1050e-12 2.8570e-08 1.1360e-07 22 1 4.2630e-20 3.1230e-12 2.4250e-08 1.0580e-07 24 1 6.5920e-20 9.8290e-13 1.9850e-08 9.4630e-08 26 1 9.6130e-21 3.0390e-13 1.5470e-08 8.1790e-08 28 1 1.8570e-20 2.4890e-13 1.1360e-08 6.8240e-08 30 1 1.2020e-19 2.0240e-13 7.8780e-09 5.4130e-08 32 1 6.6970e-21 1.1100e-13 5.1240e-09 4.0980e-08 34 1 9.0440e-20 4.3320e-14 3.1480e-09 2.9700e-08 36 1 1.5270e-20 1.2960e-14 1.8450e-09 2.0230e-08 38 1 2.4040e-20 3.1380e-15 1.0040e-09 1.2800e-08 40 1 3.3390e-20 5.9170e-16 4.7780e-10 7.6390e-09 42 1 5.2860e-20 1.0150e-16 1.8750e-10 4.3500e-09 44 1 1.5200e-19 1.5340e-17 5.8070e-11 2.3080e-09 46 1 1.0200e-19 1.4930e-18 1.3820e-11 1.0880e-09 48 1 8.9430e-20 6.5450e-19 2.7130e-12 4.3630e-10 50 1 4.3470e-20 5.1020e-21 7.2430e-13 1.4350e-10 52 1 3.9810e-20 2.1610e-19 3.6890e-13 3.7210e-11 54 1 1.6520e-19 3.9130e-20 1.9470e-13 7.1150e-12 56 1 1.5900e-20 1.5550e-21 8.2410e-14 8.6280e-13 58 1 2.1410e-19 1.9250e-19 2.8400e-14 6.0590e-14 60 1 3.1630e-20 2.4120e-20 8.1390e-15 3.6890e-14 62 1 2.7760e-20 5.9390e-21 1.9940e-15 3.3280e-14 64 1 7.3180e-20 1.3720e-19 4.3740e-16 1.7120e-14 66 1 1.4420e-19 1.3220e-19 8.9350e-17 6.4420e-15 68 1 1.2750e-19 3.4930e-19 1.3920e-17 1.9090e-15 70 1 1.1020e-19 5.9950e-20 3.1070e-18 4.8810e-16 72 1 5.1230e-20 4.0390e-20 2.1530e-19 1.1610e-16 74 1 1.7170e-20 2.8530e-20 5.6550e-20 2.0250e-17 76 1 1.1360e-19 1.7260e-20 1.7310e-20 4.8070e-18 78 1 3.4350e-19 2.1250e-19 1.5650e-19 3.6820e-19 0 2 4.9770e-13 3.7470e-11 2.7770e-08 6.6770e-08 2 2 7.8580e-12 2.9270e-10 1.4080e-07 3.3200e-07 4 2 1.3800e-11 3.8840e-10 2.4290e-07 5.8580e-07 6 2 6.0020e-12 5.1570e-10 3.3870e-07 8.2420e-07 8 2 1.2350e-12 6.3620e-10 4.1360e-07 1.0320e-06 10 2 1.5130e-13 4.5990e-10 4.7200e-07 1.2150e-06 12 2 1.2580e-14 5.9610e-10 5.0890e-07 1.3510e-06 14 2 7.5360e-16 4.6910e-10 5.1850e-07 1.4530e-06 16 2 4.0060e-17 3.0000e-10 5.1180e-07 1.5000e-06 18 2 3.2680e-19 3.5250e-10 4.7880e-07 1.5020e-06 20 2 1.4930e-19 3.4650e-10 4.3040e-07 1.4600e-06 22 2 2.2850e-20 2.3630e-10 3.7120e-07 1.3650e-06 24 2 5.1840e-20 1.3660e-10 3.0250e-07 1.2400e-06 26 2 2.6050e-19 7.5470e-11 2.3420e-07 1.0840e-06 28 2 1.4630e-19 3.7740e-11 1.7070e-07 9.0370e-07 30 2 1.5650e-19 1.5770e-11 1.1570e-07 7.2380e-07 32 2 1.1540e-20 5.3510e-12 7.3510e-08 5.5160e-07 34 2 5.1210e-20 1.4840e-12 4.3190e-08 3.9260e-07 36 2 3.6020e-20 3.4100e-13 2.2430e-08 2.6200e-07 38 2 9.7200e-21 6.6170e-14 1.0100e-08 1.6540e-07 40 2 2.8650e-20 1.0970e-14 4.3130e-09 9.6870e-08 42 2 1.8930e-19 1.6020e-15 2.1310e-09 5.0810e-08 44 2 1.4420e-19 2.0330e-16 1.2650e-09 2.3520e-08 46 2 8.2020e-21 2.1620e-17 7.4720e-10 9.9520e-09 48 2 8.0170e-21 3.1440e-18 3.8510e-10 4.2000e-09 50 2 5.5600e-20 3.9840e-19 1.6770e-10 1.9090e-09 52 2 1.5440e-20 6.8180e-20 6.2000e-11 9.1260e-10 54 2 1.0980e-19 3.1540e-20 1.9730e-11 4.2050e-10 56 2 2.2300e-20 1.1200e-19 5.4800e-12 1.7550e-10 58 2 1.1300e-19 9.0050e-20 1.3430e-12 6.4750e-11 60 2 2.8600e-20 2.9560e-20 2.9360e-13 2.1070e-11 62 2 1.3030e-19 2.5030e-20 5.7910e-14 6.0740e-12 64 2 2.9060e-19 1.3740e-19 1.0320e-14 1.5640e-12 66 2 8.0130e-20 3.7220e-20 1.6790e-15 3.6260e-13 68 2 1.0940e-19 2.7440e-20 2.5280e-16 7.5990e-14 70 2 3.5220e-20 1.9090e-19 3.3270e-17 1.4640e-14 72 2 2.7480e-21 1.1300e-19 3.6850e-18 2.5520e-15 74 2 3.7070e-20 8.2330e-20 7.7140e-19 4.0930e-16 76 2 3.3190e-20 7.9700e-20 4.2130e-20 6.0570e-17 78 2 6.4360e-20 4.1890e-20 6.0600e-22 1.0190e-17 0 3 3.7470e-13 9.8510e-10 1.9260e-07 3.8900e-07 2 3 6.8210e-12 5.3260e-09 9.3390e-07 1.9210e-06 4 3 4.1620e-12 8.0160e-09 1.6600e-06 3.4230e-06 6 3 7.4850e-13 1.1610e-08 2.2920e-06 4.8080e-06 8 3 4.8460e-14 1.1290e-08 2.8550e-06 6.1150e-06 10 3 1.9280e-15 1.2520e-08 3.2900e-06 7.1990e-06 12 3 6.5570e-16 1.1470e-08 3.5820e-06 8.1610e-06 14 3 1.2920e-16 8.9600e-09 3.7570e-06 8.8260e-06 16 3 1.4530e-17 8.0140e-09 3.7400e-06 9.2790e-06 18 3 1.2710e-18 6.6410e-09 3.6120e-06 9.4630e-06 20 3 2.4930e-19 4.7200e-09 3.3400e-06 9.3050e-06 22 3 9.8770e-20 3.1660e-09 2.9480e-06 8.9420e-06 24 3 2.1760e-20 1.9610e-09 2.5080e-06 8.2710e-06 26 3 7.7010e-21 1.0220e-09 2.0160e-06 7.3510e-06 28 3 1.9560e-19 4.2780e-10 1.5300e-06 6.3320e-06 30 3 2.2800e-21 1.4390e-10 1.1070e-06 5.1890e-06 32 3 4.8910e-20 3.9480e-11 7.5040e-07 4.0040e-06 34 3 1.2690e-19 9.0030e-12 4.6620e-07 2.9450e-06 36 3 2.8930e-20 1.7360e-12 2.7250e-07 2.0550e-06 38 3 3.9090e-20 2.8740e-13 1.5850e-07 1.3260e-06 40 3 1.6020e-19 4.1330e-14 9.2850e-08 7.8350e-07 42 3 2.0790e-20 5.2390e-15 5.2030e-08 4.3510e-07 44 3 2.7240e-19 5.7980e-16 2.6320e-08 2.3570e-07 46 3 9.7810e-20 6.0380e-17 1.1660e-08 1.2570e-07 48 3 2.3180e-20 5.6550e-18 4.4900e-09 6.4110e-08 50 3 3.8260e-20 4.2500e-19 1.5090e-09 3.0070e-08 52 3 2.0790e-19 7.8320e-20 4.4580e-10 1.2650e-08 54 3 1.8660e-20 5.6130e-20 1.1680e-10 4.7260e-09 56 3 3.1950e-19 6.1440e-21 2.7350e-11 1.5690e-09 58 3 8.8140e-21 1.8080e-20 5.7720e-12 4.6430e-10 60 3 7.0860e-20 4.6240e-20 1.1040e-12 1.2330e-10 62 3 1.5560e-19 1.6450e-19 1.9230e-13 2.9590e-11 64 3 5.2980e-20 3.3000e-20 3.0750e-14 6.4490e-12 66 3 1.0920e-19 6.4510e-21 4.5280e-15 1.2840e-12 68 3 8.6860e-20 1.9400e-19 6.1910e-16 2.3480e-13 70 3 2.1330e-20 4.3350e-20 7.7660e-17 3.9540e-14 72 3 4.9790e-21 2.2030e-20 8.9170e-18 6.1880e-15 74 3 6.9400e-20 1.3840e-19 1.1570e-18 8.8650e-16 76 3 2.0060e-19 4.0790e-20 3.6830e-19 1.2410e-16 78 3 1.8730e-20 1.5440e-19 1.5930e-19 2.1720e-17 0 4 6.6450e-12 5.7130e-09 7.7230e-07 1.3560e-06 2 4 1.0650e-11 2.1000e-08 3.9090e-06 6.8470e-06 4 4 1.8560e-11 4.1060e-08 6.8090e-06 1.2080e-05 6 4 1.4130e-11 4.5470e-08 9.5740e-06 1.7310e-05 8 4 5.2250e-12 5.2890e-08 1.1880e-05 2.1900e-05 10 4 1.1070e-12 5.1330e-08 1.3780e-05 2.6410e-05 12 4 1.5140e-13 4.0800e-08 1.5190e-05 2.9970e-05 14 4 1.4500e-14 3.5490e-08 1.5840e-05 3.3110e-05 16 4 9.9950e-16 2.6780e-08 1.6070e-05 3.5310e-05 18 4 5.2080e-17 1.7200e-08 1.5470e-05 3.6360e-05 20 4 2.8390e-18 1.1330e-08 1.4330e-05 3.6750e-05 22 4 3.9710e-19 7.3760e-09 1.2810e-05 3.5590e-05 24 4 9.6760e-21 4.1610e-09 1.0740e-05 3.3380e-05 26 4 2.3360e-20 1.9720e-09 8.5790e-06 3.0420e-05 28 4 5.8640e-20 7.9870e-10 6.5400e-06 2.6240e-05 30 4 2.2220e-19 2.8020e-10 4.5930e-06 2.1470e-05 32 4 1.0380e-19 8.5050e-11 2.9490e-06 1.6850e-05 34 4 2.8460e-20 2.2210e-11 1.8020e-06 1.2380e-05 36 4 6.3990e-20 4.9780e-12 1.0720e-06 8.3230e-06 38 4 1.7360e-19 9.5930e-13 5.9860e-07 5.1760e-06 40 4 1.3300e-19 1.6010e-13 2.9760e-07 3.0620e-06 42 4 3.8630e-19 2.3290e-14 1.2760e-07 1.7260e-06 44 4 5.3770e-20 2.9330e-15 4.6940e-08 8.9750e-07 46 4 3.1560e-21 3.3800e-16 1.5030e-08 4.1470e-07 48 4 5.0970e-19 3.9590e-17 4.3000e-09 1.6620e-07 50 4 3.2070e-19 4.8610e-18 1.1410e-09 5.7190e-08 52 4 2.7830e-20 2.8440e-20 2.9100e-10 1.6870e-08 54 4 2.1470e-20 1.7410e-20 7.2750e-11 4.2850e-09 56 4 6.0560e-20 9.1800e-22 1.7720e-11 9.4710e-10 58 4 5.2350e-20 1.0090e-20 4.1190e-12 1.8700e-10 60 4 9.2720e-20 2.5850e-19 8.9230e-13 3.4860e-11 62 4 9.4630e-20 2.4410e-20 1.7790e-13 6.7180e-12 64 4 3.5610e-20 1.2470e-19 3.2070e-14 1.4350e-12 66 4 5.8860e-20 1.3480e-20 5.3750e-15 3.3210e-13 68 4 1.1160e-19 1.6590e-19 7.9800e-16 7.6700e-14 70 4 6.1070e-20 1.8870e-19 1.1050e-16 1.6450e-14 72 4 7.5780e-21 1.3990e-19 1.4870e-17 3.2750e-15 74 4 1.0070e-20 1.0300e-19 1.3880e-18 5.5140e-16 76 4 5.3650e-20 1.1390e-20 2.5100e-19 9.4890e-17 78 4 8.1750e-21 1.4230e-19 4.5740e-19 1.6120e-17 0 5 4.7020e-11 2.7660e-08 2.3600e-06 2.8330e-06 2 5 1.2520e-10 1.5790e-07 1.1450e-05 1.3660e-05 4 5 5.4070e-11 2.3410e-07 2.0610e-05 2.5110e-05 6 5 5.7630e-11 3.0180e-07 2.8930e-05 3.5550e-05 8 5 3.1390e-11 3.0860e-07 3.6760e-05 4.7050e-05 10 5 8.0230e-12 2.6550e-07 4.3690e-05 5.7000e-05 12 5 1.2000e-12 2.2170e-07 4.8810e-05 6.7600e-05 14 5 1.1890e-13 1.4070e-07 5.3280e-05 7.6960e-05 16 5 8.4260e-15 7.5350e-08 5.4770e-05 8.4730e-05 18 5 4.4100e-16 3.4880e-08 5.4840e-05 9.2380e-05 20 5 1.8310e-17 1.0440e-08 5.2830e-05 9.6030e-05 22 5 7.3700e-19 6.7480e-09 4.7660e-05 9.7890e-05 24 5 1.0070e-19 1.1290e-08 4.1470e-05 9.7230e-05 26 5 1.7210e-20 1.1140e-08 3.4150e-05 9.1090e-05 28 5 1.2820e-19 6.8810e-09 2.5460e-05 8.2100e-05 30 5 5.3750e-20 3.0120e-09 1.7450e-05 7.1100e-05 32 5 5.7550e-20 1.0050e-09 1.1280e-05 5.6800e-05 34 5 2.8470e-20 2.6730e-10 6.6080e-06 4.1470e-05 36 5 2.0190e-20 5.8520e-11 3.2230e-06 2.8330e-05 38 5 9.9730e-20 1.0790e-11 1.2210e-06 1.8120e-05 40 5 2.8360e-20 1.7040e-12 3.4820e-07 1.0400e-05 42 5 5.1480e-20 2.3370e-13 8.7570e-08 5.0970e-06 44 5 1.0970e-19 2.8270e-14 3.7330e-08 2.0740e-06 46 5 8.1570e-20 2.9810e-15 2.5970e-08 7.0130e-07 48 5 1.0370e-19 2.9720e-16 1.5970e-08 2.1080e-07 50 5 4.2090e-20 2.1200e-17 7.6990e-09 6.8290e-08 52 5 9.5670e-20 1.9150e-18 2.9960e-09 2.8530e-08 54 5 5.4280e-20 8.8190e-20 9.7370e-10 1.3630e-08 56 5 7.5550e-20 2.3100e-20 2.7130e-10 6.1080e-09 58 5 5.9710e-20 2.1130e-21 6.6000e-11 2.3820e-09 60 5 1.4240e-20 8.1600e-20 1.4230e-11 8.0170e-10 62 5 1.5620e-19 3.2300e-19 2.7440e-12 2.3520e-10 64 5 9.3280e-22 4.5210e-21 4.7820e-13 6.0870e-11 66 5 2.6620e-21 6.5440e-20 7.5680e-14 1.4060e-11 68 5 1.2820e-19 3.0230e-20 1.0930e-14 2.9240e-12 70 5 3.7390e-20 8.7230e-20 1.4650e-15 5.5220e-13 72 5 1.0790e-20 1.6560e-19 1.7020e-16 9.5190e-14 74 5 5.8110e-20 1.8540e-19 2.0300e-17 1.5140e-14 76 5 2.1750e-19 1.8630e-19 1.8890e-18 2.1330e-15 78 5 8.1410e-21 4.6860e-20 9.5300e-20 3.8390e-16 0 6 2.4720e-10 2.4120e-07 3.4270e-06 2.4800e-06 2 6 3.1120e-10 1.1470e-06 1.7510e-05 1.3780e-05 4 6 2.0020e-11 1.9190e-06 3.1290e-05 2.3730e-05 6 6 2.0800e-10 2.4890e-06 4.5150e-05 3.6570e-05 8 6 1.2710e-10 2.6820e-06 5.9490e-05 4.7510e-05 10 6 3.1480e-11 2.7150e-06 7.1800e-05 6.1800e-05 12 6 4.4380e-12 2.3710e-06 8.6310e-05 7.5720e-05 14 6 4.1090e-13 1.9200e-06 9.6080e-05 8.9910e-05 16 6 2.7090e-14 1.4200e-06 1.0650e-04 1.0800e-04 18 6 1.3290e-15 9.1140e-07 1.1410e-04 1.2140e-04 20 6 4.4830e-17 6.0130e-07 1.1460e-04 1.3790e-04 22 6 2.0510e-18 4.4380e-07 1.1410e-04 1.5290e-04 24 6 2.5710e-20 3.0070e-07 1.0800e-04 1.5920e-04 26 6 2.7780e-19 1.6240e-07 9.3100e-05 1.6410e-04 28 6 4.5810e-19 6.8440e-08 7.6320e-05 1.6340e-04 30 6 6.4430e-19 2.2900e-08 5.9880e-05 1.4900e-04 32 6 2.2030e-19 6.2360e-09 4.2080e-05 1.2680e-04 34 6 2.7760e-20 1.4120e-09 2.5430e-05 1.0340e-04 36 6 1.3220e-19 2.7100e-10 1.3740e-05 7.8070e-05 38 6 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